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- W2103111020 abstract "Here we present a study on the metastble decay of the deprotonated deoxynucleosides dC, dT, dA and dG. We discuss the underlying mechanisms and compare the fragmentation pattern we observe to the fragment formation observed through dissociative electron attachment. The deprotonated deoxynucleosides show characteristic decay spectra which composition is mainly governed by the nature of the base, i.e., if the deoxynucleoside contains a pyrimidine or a purine base. The deoxynucleosides containing purine decompose predominantly through the simple rupture of the glycosidic bond, leading to the observation of the negatively charged, deprotonated base [B-H]-. The only other fragment observed for dA and dG is [B+C2H2]-. The deoxynucleosides containing pyrimidine (dC and dT) show a considerably richer fragmentation pattern with one of the dominating fragments being the negative ion of the high electron affinity fragment NCO. In the case of dT all other fragments may be traced to decomposition of the sugar moiety. The fragmentation spectra of dC on the other hand are governed by the decomposition of the base." @default.
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- W2103111020 date "2008-02-01" @default.
- W2103111020 modified "2023-09-26" @default.
- W2103111020 title "Metastable decay of deprotonated deoxynucleosides in matrix assisted laser desorption/ionization." @default.
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- W2103111020 doi "https://doi.org/10.1088/1742-6596/101/1/012017" @default.
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