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- W2103121245 abstract "This study deals with the investigation of microphase-separated morphology and phase behaviour in blends of polystyrene-block-polyisoprene with homopolystyrene and blends of polystyrene-block-poly(methyl methacrylate) with homopoly(methyl methacrylate) or homopolystyrene in the strong segregation regime using small-angle X-ray scattering and transmission electron microscopy as a function of composition, molecular weight of homopolymers, rM and temperature. Parameter rM = MH/MC (where MH is the molecular weight of homopolymer and MC that of the corresponding block copolymer) was selected to encompass behaviour of the chains denoted as a ‘wet brush’ (i.e. rM < 1). The relative domain spacing D/Do increases in the regime 0 < rM⩽1 with increasing concentration of homopolymer wP and increasing rM but depends on the specific implemented morphology. We tested a new approximate D/Do versus wP relation in the strong segregation regime using block copolymers of high molecular weights. It is shown that the parameters rM and χ3/2N determine the slope of the D/Do versus wP relation in the strong segregation regime and the new approximation generally matches the experimental data better than the approximations used so far. Copyright © 2010 Society of Chemical Industry" @default.
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- W2103121245 date "2010-12-14" @default.
- W2103121245 modified "2023-10-17" @default.
- W2103121245 title "Self-assembled structures in polystyrene-block-polyisoprene-blend-polystyrene and polystyrene-block-poly(methyl methacrylate)-blend-polystyrene or -blend-poly(methyl methacrylate) in the strong segregation regime" @default.
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- W2103121245 doi "https://doi.org/10.1002/pi.2994" @default.
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