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• W2103199894 abstract "Previous time-resolved FTIR measurements suggested the involvement of an intermediary component in the electron transfer step QA- → QB in the photosynthetic reaction center (RC) from Rhodobacter sphaeroides [Remy and Gerwert (2003) Nat. Struct. Biol. 10, 637]. By a kinetic X-ray absorption experiment at the Fe K-edge we investigated whether oxidation occurs at the ferric non-heme iron located between the two quinones. In isolated reaction centers with a high content of functional QB, at a time resolution of 30 μs and at room temperature, no evidence for transient oxidation of Fe was obtained. However, small X-ray transients occurred, in a similar micro- to millisecond time range as in the IR experiments, which may point to changes in the Fe ligand environment due to the charges on QA- and QB-. In addition, VIS measurements agree with the IR data and do not exclude an intermediate in the QA- → QB transition." @default.
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• W2103199894 date "2005-12-15" @default.
• W2103199894 modified "2023-09-23" @default.
• W2103199894 title "A Time-Resolved Iron-Specific X-ray Absorption Experiment Yields No Evidence for an Fe²⁺→ Fe³⁺Transition during Q_A^-→ Q_BElectron Transfer in the Photosynthetic Reaction Center" @default.
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• W2103199894 doi "https://doi.org/10.1021/bi0515725" @default.
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