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- W2103292923 abstract "Two quaternary sulfides RE3Sb0.33SiS7 (RE=La, Pr) have been prepared from stoichiometric mixtures of elements at 1223 K in an evacuated silica tube. They are the first examples of chalcogenides in the quaternary RE/Si/Sb/Q (RE=rare earth metal; Q=S, Se, Te) system. These two isostructural materials crystallize in the Ce3Al1.67S7 structure type in the hexagonal space group P63. Their structure features one-dimensional chains of face-sharing SbS6 octahedra running parallel to the c direction surrounded by the discrete SiS4 tetrahedra and RE cations. The La3Sb0.33SiS7 exhibits a SHG signal about 0.5 times that of the commercially used IR NLO material AgGaS2 at 2.05 μm laser. The optical gap of 1.92 eV for La3Sb0.33SiS7 was deduced from UV/Vis reflectance spectroscopy." @default.
- W2103292923 created "2016-06-24" @default.
- W2103292923 creator A5022469389 @default.
- W2103292923 date "2015-07-01" @default.
- W2103292923 modified "2023-10-09" @default.
- W2103292923 title "Syntheses, crystal structures, and NLO properties of the quaternary sulfides RE3Sb0.33SiS7 (RE=La, Pr)" @default.
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- W2103292923 doi "https://doi.org/10.1016/j.jssc.2015.03.010" @default.
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