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W2103607370 abstract "(Ce x Ca 1-x )F 2+x single crystal with x = 0.0001 - 0.03 were grown by the mu-PD method. Ce 3+ doping in CaF 2 lattice gives rise to characteristic absorption and emission bands, which are governed by the characteristics of the isolated Ce 3+ -F i - C 4v pair centers and small clusters composed from these pairs. With increasing Ce concentration there is a strong increase of the absorption bands related to the cluster centres, but the radioluminescence spectra are always governed by the emission of the isolated Ce 3+ -F i - C 4v pairs without noticeable changes in the emission band shape. Highest radioluminescence intensity is achieved for Ce 0.1{%} concentration and above 1{%} of Ce the onset of concentration quenching is observed. Scintillation response is governed by the energy transfer from the CaF 2 host lattice and even for the Ce3{%} sample the dominant scintillation decay time is about 50{%} longer with respect to the photoluminescence decay time of Ce 3+ -F i - C 4v pair centres. Energy transfer processes and the role of different Ce 3+ -based centers are discussed." @default.
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W2103607370 date "2008-06-01" @default.
W2103607370 modified "2023-09-23" @default.
W2103607370 title "Single Crystal Growth and Luminescence Properties of CeF$_{3}$-CaF$_{2}$ Solid Solution Grown by the Micro-Pulling-Down Method" @default.
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W2103607370 doi "https://doi.org/10.1109/tns.2008.924091" @default.
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