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• W2103643714 abstract "A photoionization spectrometer for velocity map imaging has been developed for measuring the scattering distribution of fragment ions from polyatomic molecules. The spectrometer contains a mass gate and an ion reflector which are able to discriminate ions with a particular mass-to-charge ratio m/z . The basic functions and feasibility of these devices were tested experimentally and theoretically. First, the photoions from Kr and C 60 were extracted into a time-of-flight (TOF) mass spectrometer by a transient or continuous electrostatic field. When the pulse application on the mass gate was tuned to the arrival timing of ions with a specific m/z , the peak of the selected ions alone was present on a TOF spectrum. Second, compatibility between velocity map imaging and ion discrimination was investigated by the computer simulations of the ion trajectories of photofragments from C 60 . A pulsed voltage was applied to the mass gate synchronously with the arrival timing of <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow><mml:msub><mml:mrow><mml:mtext>C</mml:mtext></mml:mrow><mml:mrow><mml:mn mathvariant=normal>5</mml:mn><mml:mn mathvariant=normal>8</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:math> ions. The initial three-dimensional velocity distribution of <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow><mml:msub><mml:mrow><mml:mtext>C</mml:mtext></mml:mrow><mml:mrow><mml:mn mathvariant=normal>5</mml:mn><mml:mn mathvariant=normal>8</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:math> was projected onto the image plane with an energy resolution better than 10 meV. The <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow><mml:msub><mml:mrow><mml:mtext>C</mml:mtext></mml:mrow><mml:mrow><mml:mn mathvariant=normal>5</mml:mn><mml:mn mathvariant=normal>8</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:math> image was free from the contamination of other ions such as <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow><mml:msub><mml:mrow><mml:mtext>C</mml:mtext></mml:mrow><mml:mrow><mml:mn mathvariant=normal>6</mml:mn><mml:mn mathvariant=normal>0</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:math> and <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msup><mml:mrow><mml:msub><mml:mrow><mml:mtext>C</mml:mtext></mml:mrow><mml:mrow><mml:mn mathvariant=normal>5</mml:mn><mml:mn mathvariant=normal>6</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:math>." @default.
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• W2103643714 date "2012-06-26" @default.
• W2103643714 modified "2023-10-17" @default.
• W2103643714 title "Design of Velocity Map Imaging Spectrometer Equipped with a Mass Gate Discriminating Particular Photofragments" @default.
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• W2103643714 doi "https://doi.org/10.5402/2012/959074" @default.
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