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• W2103702196 abstract "A foray into the exploration of Fe analogues of the (fulvalene)tetracarbonyldiruthenium [FvRu2(CO)4] solar-thermal storage system 1 ⇆ 2 is described. It was facilitated by the development of a convenient synthetic access to the parent [FvFe2(CO)4] 3a and the more soluble di(tert-butyl)fulvalene derivatives 3c and d. Laboratory time scale irradiations (>400 nm) fail to induce photoisomerization, an observation that is explained by the results of time-resolved IR experiments. They show that photoexcitation generates only the short-lived singlet syn biradical of 3 (and a small amount of decarbonylation product), in the absence of the corresponding triplet species required for the occurrence of rearrangement to 4." @default.
• W2103702196 created "2016-06-24" @default.
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• W2103702196 date "2013-01-01" @default.
• W2103702196 modified "2023-10-16" @default.
• W2103702196 title "Switching from Ru to Fe: picosecond IR spectroscopic investigation of the potential of the (fulvalene)tetracarbonyldiiron frame for molecular solar-thermal storage" @default.
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• W2103702196 doi "https://doi.org/10.1039/c3cp51292d" @default.
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