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• W2104527393 abstract "Different density rhodium nanoparticulate substrates were fabricated by electron-beam physical vapor deposition in order to study the fluorescence of close-proximity fluorophores to the high thermally stable rhodium nanoparticles. We observed an apparently constant metal-enhanced fluorescence (MEF), when fluorophores were placed in close proximity to rhodium nanoparticles before and after autoclaving of the substrates. Fluorophores with different emission wavelength maxima and free-space quantum yields have also been studied and can undergo different enhancements, a 2.5-fold increase in far-field luminescence was observed from 15 nm Rh films for Tinopal, and up to a 10-fold enhancement was observed for fluorescein. Similarly, the near-field fluorescence enhancement values were estimated to be ∼125 and 500 fold, respectively. Further, the electromagnetic field distributions around different size Rh nanoparticles were simulated using FDTD to understand the wavelength dependence of the e-field. Our findings show that the decay time of fluorophores was not reduced near to the rhodium substrates, suggesting only an enhanced electric field component is the mechanism for fluorescence enhancement." @default.
• W2104527393 created "2016-06-24" @default.
• W2104527393 creator A5047713796 @default.
• W2104527393 creator A5050256381 @default.
• W2104527393 date "2010-01-01" @default.
• W2104527393 modified "2023-09-27" @default.
• W2104527393 title "Metal-enhanced fluorescence from thermally stable rhodium nanodeposits" @default.
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• W2104527393 doi "https://doi.org/10.1039/c0jm01806f" @default.
• W2104527393 hasPublicationYear "2010" @default.
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