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- W2105421138 startingPage "1042" @default.
- W2105421138 abstract "Two-photon-induced polarization spectroscopy of molecular nitrogen in the a1Πg(ν′ = 1) ← X1Σg+ (ν″ = 0) system near 283 nm was performed, and its signal dependence investigated over the pressure range from 1.2 to 5 bars at 300 K. A significant increase of the signal intensity with pressure beyond the expected square law for a two-photon process was observed for pure nitrogen. Similar behavior was also found for a constant nitrogen partial pressure with increasing partial pressures of argon buffer gas. In both cases the spectral linewidth of the excited transitions increased dramatically with overall pressure. A possible explanation is given for the observed behavior in terms of contributions to the nonlinear susceptibility of the medium from the population of one-photon resonantly absorbing excited-state nitrogen and ground state N2+ ions created in the multiphoton absorption process at the high laser intensities required." @default.
- W2105421138 created "2016-06-24" @default.
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- W2105421138 date "2000-02-20" @default.
- W2105421138 modified "2023-09-24" @default.
- W2105421138 title "Investigation of two-photon-induced polarization spectroscopy of the a–X (1,0) transition in molecular nitrogen at elevated pressures" @default.
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- W2105421138 doi "https://doi.org/10.1364/ao.39.001042" @default.
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