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• W2105491566 abstract "Addressing capacity fading during electrochemical cycling is one of the most challenging issues of lithium-ion batteries based on LiMn2O4. Accordingly, in this work, an ester-functionalized ionic liquid, N-methylpyrrolidinium-N-acetate bis(trifluoromethylsulfonyl) imide ([MMEPyr][TFSI]), was designed as an additive to the electrolyte employed for Li/LiMn2O4 batteries to improve their electrochemical performance. A systematic comparative study was carried out using the LiTFSI-based electrolyte with and without [MMEPyr][TFSI] additive. After 100 cycles, the Li/LiMn2O4 half-cells retained 94 % of their initial discharge capacity in the electrolyte containing 10 wt-% [MMEPyr][TFSI]. However, the cycling capacity of the half-cells in the electrolyte without [MMEPyr][TFSI] decreased considerably to ~21 mAh g–1 within the first 10 cycles. One of the main reasons for the decrease is the stabilization of the Al current collector by the [MMEPyr][TFSI] additive, as demonstrated by scanning electron microscopy, cyclic voltammetry, and Fourier transform infrared spectroscopy. Moreover, the Li/LiMn2O4 cells in the electrolyte containing [MMEPyr][TFSI] displayed high-rate performance, whereby ~90 % of the cell initial discharge capacity was retained at 2.5C." @default.
• W2105491566 created "2016-06-24" @default.
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• W2105491566 date "2015-01-01" @default.
• W2105491566 modified "2023-10-18" @default.
• W2105491566 title "Improving Cycling Performance of LiMn2O4 Battery by Adding an Ester-Functionalized Ionic Liquid to Electrolyte" @default.
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• W2105491566 doi "https://doi.org/10.1071/ch15154" @default.
• W2105491566 hasPublicationYear "2015" @default.
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