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- W2106119574 abstract "Abstract Brevetoxin A is a decacyclic ladder toxin that possesses 5‐, 6‐, 7‐, 8‐, and 9‐membered oxacycles, as well as 22 tetrahedral stereocenters. Herein, we describe a unified approach to the B, E, G, and J rings based upon a ring‐closing metathesis strategy from the corresponding dienes. The enolate technologies developed in our laboratory allowed access to the precursor acyclic dienes for the B, E, and G medium‐ring ethers. The strategies developed for the syntheses of these four monocycles ultimately provided multigram quantities of each of the rings, supporting our efforts toward the completion of a convergent synthesis of brevetoxin A." @default.
- W2106119574 created "2016-06-24" @default.
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- W2106119574 date "2009-09-03" @default.
- W2106119574 modified "2023-10-09" @default.
- W2106119574 title "Enantioselective Total Synthesis of Brevetoxin A: Unified Strategy for the B, E, G, and J Subunits" @default.
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- W2106119574 doi "https://doi.org/10.1002/chem.200900776" @default.
- W2106119574 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/2826130" @default.
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- W2106119574 hasPublicationYear "2009" @default.
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