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• W2106723391 abstract "We report a low-cost fabrication method that transforms silica paper into an array of nanopipes with conductive, nanoscopic carbon walls in which the inner and outer carbon surfaces and the inner and outer voids are interconnected in three dimensions. Ultrathin (10–800 nm) carbon coatings are controllably deposited at 1000°C from hydrocarbon vapors onto the fibers of commercial silica filter paper to create a conductive C@SiO2 paper with a shell of carbon wrapping each silica fiber. The cylindrical silica fibril cores that comprise the paper can then be chemically etched to yield a self-supported assembly of hollow, open, thin-walled carbon pipes with continuous electronic pathways and large interfacial areas while retaining the form factor of the original silica paper. Many lost-wax templating approaches have been reported, but this protocol enables one to synthetically fine-tune the carbon wall thickness in ∼10-nm increments such that the ratio of the inner diameter of the pipe to the wall thickness can be as large as 100:1. This two-step route to scalable arrays of carbon pipes (ductwork) uses inexpensive and readily available precursors and generates a freestanding ultraporous object that can function as stand-alone electrode nanoarchitectures. Such macroscale form factors with nanoscopic conductive conduits are adaptable for advanced energy-storage devices or as an ultralight matrix for thermal management such as spot cooling." @default.
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• W2106723391 date "2013-01-01" @default.
• W2106723391 modified "2023-09-23" @default.
• W2106723391 title "Carbon Ductwork with Nanometric Walls and Micron-to-Submicron Inner Diameters" @default.
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• W2106723391 doi "https://doi.org/10.1149/2.013310jss" @default.
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