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- W2107322840 abstract "The process of electron transfer between methyl viologen radicals and water in photolytic systems was investigated. It was found that upon irradiation the steady-state concentration of reduced methyl viologen was pH-dependent and that hydrogen was produced without a catalyst. Electrochemical reduction of methyl viologen showed that the radical acts as an acid-base indicator. It could be shown that the electron transfer process occurs intramolecularly via a colourless methyl viologen radical-proton complex (pKa = 4.0 ∓ 0.2). Hitherto the catalyst was believed to operate as an electron acceptor for methyl viologen radicals. Now it could be proved that the noble metal acts merely as a site for hydrogen deposition and recombination for the intramolecular reduced hydrogen atoms." @default.
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- W2107322840 date "1992-02-01" @default.
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- W2107322840 title "A new mechanism for electron transfer between methyl viologen radicals and water" @default.
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- W2107322840 doi "https://doi.org/10.1016/0304-5102(92)80031-b" @default.
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