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- W2108171688 abstract "The rhodium-catalyzed regio- and enantioselective amination of racemic tertiary allylic trichloroacetimidates with a variety of aniline nucleophiles is a direct and efficient route to chiral α,α-disubstituted allylic N-arylamines. We describe the first dynamic kinetic asymmetric transformations of racemic tertiary allylic electrophiles with anilines utilizing a chiral diene-ligated rhodium catalyst. The method allows for the formation of α,α-disubstituted allylic N-arylamines in moderate to good yields with good to excellent levels of regio- and enantioselectivity." @default.
- W2108171688 created "2016-06-24" @default.
- W2108171688 creator A5002931824 @default.
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- W2108171688 date "2012-05-14" @default.
- W2108171688 modified "2023-10-16" @default.
- W2108171688 title "Rhodium-Catalyzed Dynamic Kinetic Asymmetric Transformations of Racemic Tertiary Allylic Trichloroacetimidates with Anilines" @default.
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- W2108171688 doi "https://doi.org/10.1021/ja302223p" @default.
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