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- W2108538165 abstract "We present results of large-scale molecular dynamics simulations of hard sphere systems at values of the volume fraction $ensuremath{varphi}$ along the disordered, metastable branch of the phase diagram up to random close-packing ${ensuremath{varphi}}_{c}$. By quantifying the degree of local order, we determine the necessary conditions to obtain a truly random system, enabling us to compute the pressure carefully along the entire metastable branch. Near ${ensuremath{varphi}}_{c}$ we show that the pressure scales as $({ensuremath{varphi}}_{c}ensuremath{-}ensuremath{varphi}{)}^{ensuremath{-}ensuremath{gamma}}$, where $ensuremath{gamma}phantom{rule{0ex}{0ex}}=phantom{rule{0ex}{0ex}}1$ and ${ensuremath{varphi}}_{c}phantom{rule{0ex}{0ex}}=phantom{rule{0ex}{0ex}}0.644ifmmodepmelsetextpmfi{}0.005$. Contrary to previous studies, we find no evidence of a thermodynamic glass transition and find that after long times the system crystallizes for all $ensuremath{varphi}$ above the melting point." @default.
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- W2108538165 date "1996-11-11" @default.
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- W2108538165 title "Metastability and Crystallization in Hard-Sphere Systems" @default.
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- W2108538165 doi "https://doi.org/10.1103/physrevlett.77.4198" @default.
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