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• W2108682309 abstract "The structural phase transition of gadolinium–scandium–gallium garnet (Gd3Sc2Ga3O12, GSGG) has been studied at high pressure and high temperature using the synchrotron X-ray diffraction technique in a laser-heated diamond anvil cell. The GSGG garnet transformed to an orthorhombic perovskite structure at approximately 24 GPa after laser heating to 1500–2000 K. The garnet-to-perovskite phase transition is associated with an ∼8% volume reduction and an increase in the coordination number of the Ga3+ or Sc3+ ion. The orthorhombic perovskite GSGG has bulk modulus B0 = 194(15) GPa with B0′ = 5.3(8), exhibiting slightly less compression than the cubic garnet structure of GSGG with B0 = 157(15) GPa and B0′ = 6.5(10). Upon compression at room temperature, the cubic GSGG garnet became amorphous at ∼65 GPa. Coupled with the amorphous-to-perovskite phase transition in Y3Fe5O12 and Gd3Ga5O12 at high-pressure–temperature conditions, we conclude that amorphization should represent a new thermodynamic state resulting from hindrance of the garnet-to-perovskite phase transition, whereas the garnet-to-amorphous transition in rare-earth garnets should be kinetically hindered at room temperature." @default.
• W2108682309 created "2016-06-24" @default.
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• W2108682309 date "2012-12-14" @default.
• W2108682309 modified "2023-09-22" @default.
• W2108682309 title "Garnet-to-Perovskite Transition in Gd₃Sc₂Ga₃O₁₂ at High Pressure and High Temperature" @default.
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• W2108682309 doi "https://doi.org/10.1021/ic302245x" @default.
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