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• W2108698596 abstract "Experiments were performed to determine the equilibrium as well as kinetic stable nitrogen and oxygen isotope fractionations between aqueous dissolved and gaseous N2O. The equilibrium fractionations, defined as the ratio of the isotopic abundance ratios (15R and 18R, respectively) of gaseous and dissolved N2O were found to be 0.99925 for 15N14N and 0.99894 for 18O16O at 298.2 K. No temperature dependence could be observed over the temperature range of 273.2–317.7 K outside experimental error. At 298.2 K the kinetic fractionation factors during N2O invasion (15αin = 15R(invaded)15R(gas), and 18αin defined similarly) were 1.0000 and 0.9992, respectively, and during N2O evasion (15αev = 15R(evaded)15R(aq.solution) and 18αev defined similarly) were 0.9993 and 0.9981, respectively. The resulting changes in δ-values during air to sea transfer of N2O are 0.0 and −0.8‰, and for sea to air transfer −0.7 and −1.9‰, for N and O, respectively. These results are in agreement with the hypothesis that the oceans would be a large source for N2O in the atmosphere considering the fact that 15δ and 18δ of dissolved N2O were found to be slightly heavier than those in air." @default.
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• W2108698596 date "1994-03-01" @default.
• W2108698596 modified "2023-10-17" @default.
• W2108698596 title "Equilibrium and kinetic nitrogen and oxygen isotope fractionations between dissolved and gaseous N2O" @default.
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• W2108698596 doi "https://doi.org/10.1016/0009-2541(94)90009-4" @default.
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