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- W2108804476 abstract "We use a combination of R-matrix and hyperspherical coordinate techniques to study the effects of electron correlations in atomic valence shells. The 3snd-3${p}^{2}$ mixing in Mg $^{1}mathrm{D}^{mathrm{e}}$ is analyzed in detail and its relevance to the ${s}^{2}$${p}^{n}$d-${mathrm{sp}}^{n+2}$ interactions throughout the row is indicated by a study of the 3${s}^{2}$nd-3s3${p}^{2}$ ${}^{2}$${D}^{e}$ mixing in Al. Multichannel quantum-defect theory parameters for Mg $^{1}mathrm{D}^{mathrm{e}}$ and Al $^{2}mathrm{D}^{mathrm{e}}$ are calculated ab initio. We obtain excellent agreement with experiment for the quantum defects of the 3snd series in Mg and a significant improvement over previous theoretical studies for the quantum defects of the 3${s}^{2}$nd series in Al. Two-electron correlations are illustrated by mapping their joint probability density for alternative eigenmodes." @default.
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- W2108804476 title "Electron correlations in atomic valence shells: Magnesium and aluminum" @default.
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- W2108804476 doi "https://doi.org/10.1103/physreva.32.908" @default.
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