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• W2109191528 abstract "Caloric curves for sodium clusters with N=139 and 147 atoms show a fine structure near the solid-to-liquid transition. Neither of the two sizes exhibit surface melting. For N=139, diffusion of the surface vacancies is observed, which is not possible in the closed-shell N=147 cluster. A few kelvin above the peak in the heat capacity, N=139 is completely liquid. This is not the case for N=147. Here the inner 13 atoms remain nearly fixed up to several tens of kelvin above the melting temperature of the outer two layers. A simple physical reason is suggested for this unexpected behavior." @default.
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• W2109191528 date "2009-01-29" @default.
• W2109191528 modified "2023-09-27" @default.
• W2109191528 title "Premelting and Postmelting in Clusters" @default.
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• W2109191528 doi "https://doi.org/10.1103/physrevlett.102.043401" @default.
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