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• W2109194245 abstract "Depending on the localization of hydroxyl groups on MgO surface irregularities, their topology and coordination can differ. In order to discriminate their reactivity, three MgO samples with different morphologies are hydroxylated at various levels. From 1H MAS NMR three kinds of OH groups can be distinguished. It is shown that the catalytic activity of base sites in the conversion of 2-methylbut-3-yn-2-ol is governed by species giving a 1H NMR signal at δ < −0.7 ppm, assigned to low coordinated O1CH and O2CH formed by water dissociation on steps and corners. Their reactivity is discussed considering charge and orbital analysis from DFT." @default.
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• W2109194245 date "2009-11-15" @default.
• W2109194245 modified "2023-10-16" @default.
• W2109194245 title "Identification of the OH groups responsible for kinetic basicity on MgO surfaces by 1H MAS NMR" @default.
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• W2109194245 doi "https://doi.org/10.1016/j.jcat.2009.09.003" @default.
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