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- W2109554425 abstract "Abstract 1‐Formyl‐19‐oxobilin‐type tetrapyrroles are characteristic, abundant products of chlorophyll breakdown in senescent leaves. However, in some leaves, 1,19‐dioxobilin‐type chlorophyll catabolites (DCCs) lacking the formyl group accumulate instead. A P450 enzyme was identified in in vitro studies that removed the formyl group of a primary fluorescent chlorophyll catabolite ( p FCC) and generated fluorescent DCCs. These DCCs are precursors of isomeric nonfluorescent DCCs (NDCCs). Here, we report a structural investigation of the NDCCs in senescent leaves of wild‐type Arabidopsis thaliana. Four new NDCCs were characterized, two of which carried a stereoselectively added hydroxymethyl group. Such formal DCC hydroxymethylations were previously found in DCCs in leaves of a mutant of A. thaliana . They are now indicated to be a feature of chlorophyll breakdown in A. thaliana , associated with the specific in vivo deformylation of p FCC en route to NDCCs." @default.
- W2109554425 created "2016-06-24" @default.
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- W2109554425 date "2015-07-14" @default.
- W2109554425 modified "2023-10-18" @default.
- W2109554425 title "Hydroxymethylated Dioxobilins in Senescent<i>Arabidopsis thaliana</i>Leaves: Sign of a Puzzling Biosynthetic Intermezzo of Chlorophyll Breakdown" @default.
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- W2109554425 doi "https://doi.org/10.1002/chem.201501489" @default.
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