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• W2109586446 abstract "Styrene radiation grafted ETFE based proton conducting membranes are subject to degradation under fuel cell operating conditions and show a poor stability. Lifetimes exceeding 250 h can only be achieved with crosslinked membranes. In this study, a novel approach based on the increase of the intrinsic oxidative stability of uncrosslinked membranes is reported. Hence, the co-grafting of styrene with methacrylonitrile (MAN), which possesses a protected α-position and strong dipolar pendant nitrile group, onto 25 μm ETFE base film was investigated. Styrene/MAN co-grafted membranes were compared to a styrene based membrane in durability tests in single H2/O2 fuel cells. It is shown that the incorporation of MAN considerably improves the chemical stability, yielding fuel cell lifetimes exceeding 1000 h. The membrane preparation based on the co-grafting of styrene and MAN offers the prospect of tuning the MAN content and introduction of a crosslinker to enhance the oxidative stability of the resulting fuel cell membranes." @default.
• W2109586446 created "2016-06-24" @default.
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• W2109586446 date "2009-05-01" @default.
• W2109586446 modified "2023-09-26" @default.
• W2109586446 title "Novel ETFE based radiation grafted poly(styrene sulfonic acid-co-methacrylonitrile) proton conducting membranes with increased stability" @default.
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• W2109586446 doi "https://doi.org/10.1016/j.elecom.2009.02.047" @default.
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