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• W2109761005 abstract "Effects of ion-exchanged alkali metal cations on the adsorption and the photolysis (Norrish type I and type II reactions) of n-butyrophenone included within the alkali metal cation-exchanged ZSM-5 zeolite have been investigated by experimental and theoretical approaches. The yields of the photolysis decreased and the ratio of the type I/type II reactions increased, respectively, by changing the ion-exchanged cations from Cs + to Li + . The observed IR spectra of the adsorbed n-butyrophenone and the ab initio molecular orbital calculations of this host–guest system indicate that the n-butyrophenone mainly interacts with alkali metal cation, while the electrostatic interaction between the n-butyrophenone and cation increases by changing the cations from Cs + to Li + . These results indicate that the smaller cation has the stronger electrostatic interaction between n-butyrophenone and promotes the Norrish type I reaction in the photolysis of n-butyrophenone. © 2003 Elsevier Science B.V. All rights reserved." @default.
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• W2109761005 date "2003-08-01" @default.
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• W2109761005 title "Experimental study and ab initio molecular orbital calculation on the photolysis of n-butyrophenone included within the alkali metal cation-exchanged ZSM-5 zeolite" @default.
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• W2109761005 doi "https://doi.org/10.1016/s1010-6030(03)00218-1" @default.
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