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• W2109889909 abstract "Controlling the structure and morphology of porous electrode materials is an effective strategy for realizing a high surface area and efficient paths for ion diffusion. Moreover, excellent electrical conductivity can significantly decrease the internal resistance of an electrode by the formation of a conductive network and facilitate the application of electrostatic charges, which favors the accumulation of an electrical double layer. In light of these facts, we demonstrate the fabrication of β-polytype porous silicon carbide spheres (PSiCS) with a hierarchical pore structure in which micro- and mesopores are interconnected with a mesoporous network. Further, to investigate the effects of the electrolyte on the electrochemical and dynamic behavior, two-electrode symmetrical supercapacitors based on the PSiCS electrode with an aqueous electrolyte (1 M potassium chloride, KCl) or an organic electrolyte (1 M tetraethylammonium tetrafluoroborate in acetonitrile, TEABF4/AN) were assembled. The symmetrical supercapacitor based on the PSiCS electrode with the aqueous electrolyte exhibited a high charge-storage capacity with a specific capacitance of 82.9 F g(-1) at a scan rate of 5 mV s(-1), which is much higher than that obtained using the organic electrolyte (60.3 F g(-1) at a scan rate of 5 mV s(-1)). However, the energy density of the organic electrolyte system was 102.59 W h kg(-1) at a scan rate of 5 mV s(-1), which is greatly superior to that of the aqueous electrolyte system (energy density: 29.47 W h kg(-1)) owing to the wide cell operating voltage range." @default.
• W2109889909 created "2016-06-24" @default.
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• W2109889909 date "2015-01-01" @default.
• W2109889909 modified "2023-09-25" @default.
• W2109889909 title "Effects of different electrolytes on the electrochemical and dynamic behavior of electric double layer capacitors based on a porous silicon carbide electrode" @default.
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• W2109889909 doi "https://doi.org/10.1039/c5cp01728a" @default.
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• W2109889909 hasPublicationYear "2015" @default.
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