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- W2110033477 abstract "Results of Monte Carlo calculations of order parameter profiles of lipid chains interacting with cholesterol are presented. Cholesterol concentrations in the simulations are sufficiently large that it is possible to analyze profiles for chains which are near neighbors of two or more cholesterol molecules, chains which are neighbors to a single cholesterol, and chains which are not near any cholesterol molecules. The profiles, show that cholesterol acts to significantly decrease the ability of neighboring chains to undergo trans-gauche isomeric rotations, although these chains are not all forced into all-trans conformations. The effect is significantly greater for chains which are neighbors to more than one cholesterol. The Monte Carlo results are next used as a guide to develop a theoretical model for lipid-cholesterol mixtures. The properties of this model and the phase diagram which it predicts are described. The phase diagram is then compared with experimentally determined phase diagrams. The model calculations and the computer simulations upon which they are based yield a molecular mechanism for several of the observed phases exhibited by lipid-cholesterol mixtures. The theoretical model predicts that at low temperatures the system should exhibit solid phase immiscibility." @default.
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- W2110033477 date "1991-02-01" @default.
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- W2110033477 title "Lipid-cholesterol interactions. Monte Carlo simulations and theory" @default.
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- W2110033477 doi "https://doi.org/10.1016/s0006-3495(91)82238-x" @default.
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