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• W2110119969 abstract "The synthesis of a vinylsulfide‐containing hydroxy acid (VSHA) from undecylenic fatty acid via thiol‐yne monoaddition is described. Metal‐ and enzymatic‐catalyzed polycondensation of VSHA is investigated to obtain functional polyesters with a view to further modification. Higher molecular weights are obtained when using enzymatic polymerization. Random copolymers are prepared by direct enzymatic copolymerization of VSHA and ε‐caprolactone (CL) and triblock CL‐VSHA‐CL copolymers are obtained by consecutive VSHA self‐condensation and ring‐opening polymerization. The copolymers display semicrystalline behavior and a good thermal stability with no significant weight loss below 300 °C. Thiol‐ene chemistry‐type crosslinking and surface functionalization are employed to open new application fields. Evidence of the successful reactions is obtained by NMR, IR, and fluorescence measurements. image" @default.
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• W2110119969 date "2014-07-14" @default.
• W2110119969 modified "2023-10-17" @default.
• W2110119969 title "Vinylsulfide-Containing Polyesters and Copolyesters from Fatty Acids: Thiol-yne Monomer Synthesis and Thiol-ene Functionalization" @default.
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• W2110119969 doi "https://doi.org/10.1002/macp.201400191" @default.
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