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- W2110592823 abstract "This chapter discusses aerobic oxidation of alcohols. The transformation of alcohols into aldehydes and ketones is of paramount importance in organic chemistry, both for laboratory-scale experiments and in the manufacturing processes. During the establishment of the scope and limitations of a useful catalytic process, some mechanistic studies are performed that allow proposing a plausible catalytic cycle, rationalizing our observations. It is remarkable that essentially every type of alcohol is smoothly oxidized into the corresponding carbonyl derivative in high yield and with good to complete conversion. Under these conditions, primary aliphatic, allylic, and benzylic alcohols afford the expected aldehydes, and secondary alcohols are smoothly transformed into ketones. Whereas, the decay of the alcohol follows the expected kinetic course, the formation of the aldehyde shows an abnormal behavior. In the early part of the reaction, the aldehyde formation matches almost perfectly the disappearance of the alcohol." @default.
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- W2110592823 date "2004-01-01" @default.
- W2110592823 modified "2023-10-18" @default.
- W2110592823 title "EFFICIENT, ECOLOGICALLY BENIGN, AEROBIC OXIDATION OF ALCOHOLS" @default.
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- W2110592823 doi "https://doi.org/10.1016/s0898-8838(04)56007-5" @default.
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