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- W2110835462 abstract "Abstract 1. (1) The subject matter of courses in electrochemistry at universities in western countries is incompatible with (a) the nature of the subject (interfacial charge transfer); (b) the extent to which electrochemical considerations play a part in surface phenomena in chemistry, metallurgy, and biology. 2. (2) What is called electrochemistry could with advantage be limited to material corresponding with the following definition: Electrochemistry is the field dealing with the relations between the passage of electric currents across interfaces and chemical surface reactions (such as a field is sometimes called electrodics). Ionics, the study of the behavior of ionic charges in condensed phases, might with advantage be taught as a part of the physical chemistry of solutions. The basic concepts of the effects of potential differences at interfaces, and the rate of charge transfer accross them, together with an outline of the basic principles of electrocatalysis, the conversion of chemical energy to electricity, and the electrochemical control of the stability of surfaces, should be a part of undergraduate courses in physical chemistry. Having regard to the many areas, the basis of which is given by such material. some half of the time on heterogeneous reactions should be used to describe interfacial electron transfer reactions. 3. (3) The basis treatment of electron transfer at interfaces was made in 1931 by Gurney. It was one of the first applications of quantum mechanics to chemistry. The treatment was misunderstood and hence neglected. 4. (4) Electrochemical reactions must always be treated quantally. 5. (5) Some chemical surface reactions have fuel cell-like mechanisms, i.e., consist of two partial reactions each of which involved electron transfer. It is speculated that such reactions may constitute the origin of currents observed in the brain." @default.
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- W2110835462 date "1968-11-01" @default.
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- W2110835462 title "A need for changes, particularly the introduction of quantum mechanical treatments, into the University teaching of electrochemistry" @default.
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- W2110835462 doi "https://doi.org/10.1016/0013-7480(68)90117-4" @default.
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