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- W2111751546 abstract "The microstructural evolution and grain-boundary influence on electrical properties of Ce0.90Gd0.10O1.95 were studied. The nanoscale powders synthesized from a semibatch reactor exhibited 50% green density and 92% sintering density at 1200°C (∼200°C lower than previous studies). Impedance spectra as a function of temperature and grain size were analyzed. The Ce0.90Gd0.10O1.95 with finest grain size possessed highest overall grain-boundary resistance; this contribution was eliminated at temperatures >600°C, regardless of grain size. The grain conductivity was independent of grain size and was dependent on temperature with two distinct regimes, indicative of the presence of Gd′Ce−Vo∘∘ complexes that dissociated at a critical temperature of ∼580°C. The activation energy for complex dissociation was ∼0.1 eV; the value for the grain-boundary was ∼1.2eV, which was size independent." @default.
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- W2111751546 date "2004-12-20" @default.
- W2111751546 modified "2023-10-14" @default.
- W2111751546 title "Microstructure and Grain-Boundary Effect on Electrical Properties of Gadolinium-Doped Ceria" @default.
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- W2111751546 doi "https://doi.org/10.1111/j.1151-2916.2002.tb00349.x" @default.
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