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• W2111778911 abstract "Decahedral morphology, with re-entrant surface modifications, is one of the common structures observed in nanoparticles. These motifs, although thermodynamically stable only at very small size ranges, have been experimentally observed to grow up to much larger sizes (100 nm to several micrometers). Whereas the surface energy plays an important role, the contributions of the elastic strain energy are nonnegligible at larger sizes and the effect of stress relaxation due to re-entrant surface faceting is poorly understood. In this article, the volumetric strain energy due to the disclination defect is computed using finite element analysis and the relaxation due to the formation of re-entrant surfaces is shown. Contrary to conventional wisdom, the disclination strain energy is shown to be a nontrivial function of the geometry and in general increases with increasing aspect ratio. The computed strain energies also result in approximately 50% increase in the stability regime than the previously reported results obtained using thermodynamical analysis. Finally, finite element analyses are utilized to explain the commonly observed defect configurations and compute the internal rigid body rotations in these particles." @default.
• W2111778911 created "2016-06-24" @default.
• W2111778911 creator A5037073937 @default.
• W2111778911 creator A5063813038 @default.
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• W2111778911 date "2013-01-14" @default.
• W2111778911 modified "2023-09-25" @default.
• W2111778911 title "Elastic Strain Energy Effects in Faceted Decahedral Nanoparticles" @default.
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• W2111778911 doi "https://doi.org/10.1021/jp310045g" @default.
• W2111778911 hasPublicationYear "2013" @default.
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