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• W2111878240 abstract "Around 0.5 K, the entropy of the spin ice $text{Dy}{}_{text{2}}{text{Ti}}_{text{2}}{text{O}}_{text{7}}$ has a plateaulike feature close to Pauling's residual entropy derived originally for water ice, but an unambiguous quantification towards lower temperature is prevented by ultraslow thermal equilibration. Based on the specific-heat data of $({text{Dy}}_{1ensuremath{-}x}{text{Y}}_{x}{)}_{text{2}}{text{Ti}}_{text{2}}{text{O}}_{text{7}}$ we analyze the influence of nonmagnetic dilution on the low-temperature entropy. With increasing $x$, the ultraslow thermal equilibration rapidly vanishes, the low-temperature entropy systematically decreases, and its temperature dependence strongly increases. These data suggest that a nondegenerate ground state is realized in $({text{Dy}}_{1ensuremath{-}x}{text{Y}}_{x}{)}_{text{2}}{text{Ti}}_{text{2}}{text{O}}_{text{7}}$ for intermediate dilution. This contradicts the expected zero-temperature residual entropy obtained from a generalization of Pauling's theory for dilute spin ice, but is supported by Monte Carlo simulations." @default.
• W2111878240 created "2016-06-24" @default.
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• W2111878240 date "2015-11-05" @default.
• W2111878240 modified "2023-09-27" @default.
• W2111878240 title "Suppression of Pauling's residual entropy in the dilute spin ice<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi>Dy</mml:mi><mml:mrow><mml:mn>1</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi mathvariant=normal>Y</mml:mi><mml:mi>x</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>Ti</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi …" @default.
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• W2111878240 doi "https://doi.org/10.1103/physrevb.92.180405" @default.
• W2111878240 hasPublicationYear "2015" @default.
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