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- W2112597660 abstract "Femtosecond photon echo, chirped four-wave mixing and pump-probe experiments are reported, using a 13 fs cavity-dumped Ti:sapphire laser for excitation. It is shown that the optical dynamics of HITCI in ethylene glycol occurs on distinctly different time scales. The ultrafast solvent response is modelled by a non-Markovian solvent oscillator, while the slow diffusional solvent motions are represented by an overdamped Markovian oscillator. With this model an oscillator-bath time correlation function is obtained that exhibits a bimodal behaviour: an initial fast Gaussian decay is followed by a slower, long exponential tail." @default.
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- W2112597660 date "1994-07-01" @default.
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- W2112597660 title "Ultrafast optical dynamics of HITCI in ethylene glycol. A non-Markovian Brownian oscillator description" @default.
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- W2112597660 doi "https://doi.org/10.1016/0009-2614(94)00559-1" @default.
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