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• W2112824746 abstract "Single crystals of YbOs2Al10 and LuOs2Al10 were grown for the first time using an aluminum self-flux method. The compounds crystallized into a cagelike structure in space group Cmcm, similar to the prototype compound YbFe2Al10. YbOs2Al10 exhibited a mixed-valent nature, as determined by magnetic susceptibility measurements over a wide temperature range from 2 to 900 K, in which the inter–configuration–fluctuation model revealed a broad peak around 400 K. In contrast, LuOs2Al10 displayed Pauli-like paramagnetic behavior over the same temperature range. Both compounds were metallic in nature between 2 and 300 K. The electronic specific heat coefficient of 21.3(2) mJ mol–1 K–2 for YbOs2Al10 was determined to be larger than that for LuOs2Al10 [8.9(1) mJ mol–1 K–2], reflecting the mixed-valent nature of the former. First-principles calculations predicted the presence of a mixed-valent state in YbOs2Al10, in agreement with the experimental observations. The novel compound YbOs2Al10 elucidates the evolution of the mixed-valent nature of the Yb-based ternary transition metal aluminides from the 3d to 5d elements." @default.
• W2112824746 created "2016-06-24" @default.
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• W2112824746 date "2014-04-21" @default.
• W2112824746 modified "2023-09-27" @default.
• W2112824746 title "Crystal Growth, Structural, Electrical, and Magnetic Properties of Mixed-Valent Compounds YbOs₂Al₁₀ and LuOs₂Al₁₀" @default.
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• W2112824746 doi "https://doi.org/10.1021/ic403168v" @default.
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