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- W2113256024 abstract "Cp 2 ZrCl 2 confined inside the supercage of NaY zeolites [NaY/methylaluminoxane (MAO)/Cp 2 ZrCl 2 ] exhibited the shape and diffusion of a monomer-controlled copolymerization mechanism that strongly depended on the molecular structure of the monomer and its size. For the ethylene-propylene copolymerization, NaY/MAO/ Cp 2 ZrCl 2 showed the effect of the comonomer on the increase in the polymerization rate in the presence of propylene, whereas the ethylene/1-hexene copolymerization showed little comonomer effect, and the ethylene/1-octene copolymerization instead showed a comonomer depression effect on the polymerization rate. Isobutylene, having a larger kinetic diameter, had little influence on the copolymerization behaviors with NaY/ MAO/Cp 2 ZrCl 2 for the ethylene-isobutylene copolymerization, which showed evidence of the shape and diffusion of a monomer-controlled mechanism. The content of the comonomer in the copolymer chain prepared with NaY/MAO/Cp 2 ZrCl 2 decreased by about one-half in comparison with that of Cp 2 ZrCl 2 . A differential scanning calorimetry study on the melting endotherms after the successive annealing of the copolymers showed that the copolymers of NaY/MAO/Cp 2 ZrCl 2 had narrow comonomer distributions, whereas those of homogeneous Cp 2 ZrCl 2 were broad." @default.
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- W2113256024 date "2003-06-06" @default.
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- W2113256024 title "Shape and diffusion of the monomer-controlled copolymerization of ethylene and ?-olefins over Cp2ZrCl2 confined in the nanospace of the supercage of NaY" @default.
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- W2113256024 doi "https://doi.org/10.1002/pola.10762" @default.
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