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- W2113337368 abstract "Quantum calculations are reported for He atoms in a gaseous mixture involving the nonlinear polyatomic system CH4. The helium-methane interaction was taken from earlier crossed beam studies [11] and the cross-sections were computed with two different coupling schemes for the angular momenta of the tensorial basis: close coupling at low energies and coupled states up to 3500 cm-1. Results for various coefficients are compared and extrapolation methods are discussed for extending them to higher temperatures. A final comparison between measured diffusion coefficients, measured mixture viscosities and the present calculations shows unequivocally that fairly realistic results can be obtained for the calculated transport properties of larger polyatomics. To the author's knowledge, it is the first time that such a comparison has been discussed using rigorous quantum methods for a mixture containing a nonlinear molecular partner." @default.
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- W2113337368 date "1995-02-20" @default.
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- W2113337368 title "Quantum calculations of transport and relaxation properties for the helium-methane system" @default.
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- W2113337368 doi "https://doi.org/10.1080/00268979500100331" @default.
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