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• W2113470578 abstract "Methyldioxorhenium (MDO)-catalyzed CO bond cleavage of a variety of lignin β-O-4-model compounds yields phenolic and aldehydic compounds in homogeneous phase under mild reaction conditions. MDO is in situ generated by reduction of methyltrioxorhenium (MTO) and is remarkably stable under the applied reaction conditions allowing its reuse for least five times without significant activity loss. Based on the observed and isolated intermediates, 17 O- and 2 H-isotope labeling experiments, DFT calculations, and several spectroscopic studies, a reaction mechanism is proposed." @default.
• W2113470578 created "2016-06-24" @default.
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• W2113470578 date "2014-01-21" @default.
• W2113470578 modified "2023-10-01" @default.
• W2113470578 title "Cleavage of CO Bonds in Lignin Model Compounds Catalyzed by Methyldioxorhenium in Homogeneous Phase" @default.
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• W2113470578 doi "https://doi.org/10.1002/cssc.201300918" @default.
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