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- W2113651435 abstract "Coherent multidimensional vibrational spectroscopy is a new technique for establishing correlations between features in vibrational spectra that are caused by intra- and intermolecular interactions. These interactions cause cross-peaks between vibrational transitions that reflect the coupling. In this paper, we use Doubly Vibrationally Enhanced Infrared Spectroscopy (DOVE-IR) and DOVE-Raman processes to obtain coherent two dimensional vibrational spectra. The spectra are fitted to obtain the dephasing rates and third order susceptibilities <TEX>$(χ^{(3)})$</TEX> for the nonlinear processes. We show that the DOVE <TEX>$χ^{(3)}$</TEX> values are directly related to the molar absorptivities and Raman <TEX>$χ^{(3)}$</TEX>. We then use these relationships to obtain estimates for the <TEX>$χ^{(3)}$</TEX> of the stimulated photon echo and <TEX>$χ^{(5)}$</TEX> of the six wave mixing spectroscopies, respectively. We also predict the ratio of the cascaded four wave mixing signal to the six wave mixing signal." @default.
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- W2113651435 date "2003-08-20" @default.
- W2113651435 modified "2023-10-16" @default.
- W2113651435 title "Experimental Determinations of Coherent Multidimensional Vibrational Spectroscopy" @default.
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- W2113651435 doi "https://doi.org/10.5012/bkcs.2003.24.8.1119" @default.
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