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• W2113706377 abstract "The steam reforming reaction of methane to synthesis gas (CO and H2) was investigated in a very broad steam-to-carbon (S/C) ratio range (0.2–7.1) over a Ni/NiAl2O4 catalyst at 843, 858, and 873 K. The dataset includes 179 data points at each temperature giving a detailed insight in the gradual change of kinetic orders in both methane and steam with changing S/C ratios as well as with total reactant partial pressures at differential conversion levels. At low S/C ratios, steam dominates the kinetics with high kinetic orders (low for methane) and vice versa for methane at high S/C ratios. The extent of the water gas shift reaction was assessed by 13CO2 co-feed experiments and thermodynamic modelling and found to be not in equilibrium. A change in the kinetic isotope effect (i.e., inverse and normal), as well as the apparent activation energy, was observed depending on the applied S/C ratios. The experimental data were satisfactorily described by a Langmuir–Hinshelwood expression." @default.
• W2113706377 created "2016-06-24" @default.
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• W2113706377 date "2014-05-23" @default.
• W2113706377 modified "2023-10-09" @default.
• W2113706377 title "Methane Steam Reforming over a Ni/NiAl₂O₄Model Catalyst-Kinetics" @default.
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• W2113706377 doi "https://doi.org/10.1002/cctc.201402017" @default.
• W2113706377 hasPublicationYear "2014" @default.
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