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• W2114850709 abstract "Polynitrogen (PN) species (Nn , n from 3 to 8) as highly energetic materials have attracted many theoretical calculations and predictions. N3 , N4 , N5 or their ions were experimentally detected under high-pressure and high-temperature conditions. Herein, a N8 (-) PN stabilized on the positively charged sidewalls of multi-walled carbon nanotubes (MWNTs) has been synthesized using cyclic voltammetry (CV) under ambient conditions. ATR-FTIR and Raman spectroscopic data assigned on the basis of density functional theory (DFT) calculations support the successful synthesis of a C2h symmetry chain structure of the N8 anion stabilized as MWNT(+) N8 (-) . Temperature programmed desorption (TPD) data show that MWNT(+) N8 (-) is thermally stable up to 400 °C. Oxygen-reduction reaction (ORR) experiments carried out using MWNT(+) N8 (-) as the cathodic catalyst shows that it is very active for ORR with an even higher current density than that of a commercial Pt/carbon catalyst." @default.
• W2114850709 created "2016-06-24" @default.
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• W2114850709 date "2014-08-14" @default.
• W2114850709 modified "2023-10-03" @default.
• W2114850709 title "N₈⁻Polynitrogen Stabilized on Multi-Wall Carbon Nanotubes for Oxygen-Reduction Reactions at Ambient Conditions" @default.
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• W2114850709 doi "https://doi.org/10.1002/anie.201403060" @default.
• W2114850709 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25123821" @default.
• W2114850709 hasPublicationYear "2014" @default.
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