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• W2115515328 abstract "The amplifying asymmetric autocatalysis discovered by Soai and coworkers in 1995 does not fit easily into the extensively investigated framework of organozinc alkylation of aldehydes. In that case the catalyst is a monomeric Zn chelate that functions as both Lewis acid and Lewis base, permitting the simultaneous coordination of both dialkylzinc reagent and aldehyde reactant. By contrast, the Soai reactants are rigid gamma-aminoaldehydes that cannot function as mononuclear chelates. Structural and computational evidence for a binuclear resting state is presented, and the energetics of mono-, di-, tri-, and tetrameric species accessible to the reacting system have been computed." @default.
• W2115515328 created "2016-06-24" @default.
• W2115515328 creator A5078065728 @default.
• W2115515328 creator A5081669336 @default.
• W2115515328 date "2004-04-01" @default.
• W2115515328 modified "2023-10-18" @default.
• W2115515328 title "Asymmetric autocatalysis: Novel structures, novel mechanism?" @default.
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• W2115515328 doi "https://doi.org/10.1073/pnas.0308178101" @default.
• W2115515328 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/395975" @default.
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