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- W2115569304 abstract "A brown mesoporous TiO2-x/MCF composite with a high fluorine dopant concentration (8.01 at%) is synthesized by a vacuum activation method. It exhibits an excellent solar absorption and a record-breaking quantum yield (Φ = 46%) and a high photon–hydrogen energy conversion efficiency (η = 34%,) for solar photocatalytic H2 production, which are all higher than that of the black hydrogen-doped TiO2 (Φ = 35%, η = 24%). The MCFs serve to improve the adsorption of F atoms onto the TiO2/MCF composite surface, which after the formation of oxygen vacancies by vacuum activation, facilitate the abundant substitution of these vacancies with F atoms. The decrease of recombination sites induced by high-concentration F doping and the synergistic effect between lattice Ti3+–F and surface Ti3+–F are responsible for the enhanced lifetime of electrons, the observed excellent absorption of solar light, and the photocatalytic production of H2 for these catalysts. The as-prepared F-doped composite is an ideal solar light-driven photocatalyst with great potential for applications ranging from the remediation of environmental pollution to the harnessing of solar energy for H2 production." @default.
- W2115569304 created "2016-06-24" @default.
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- W2115569304 date "2014-12-15" @default.
- W2115569304 modified "2023-09-26" @default.
- W2115569304 title "A Brown Mesoporous TiO<sub>2-x</sub>/MCF Composite with an Extremely High Quantum Yield of Solar Energy Photocatalysis for H<sub>2</sub>Evolution" @default.
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- W2115569304 doi "https://doi.org/10.1002/smll.201403056" @default.
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