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- W2116049076 abstract "Abstract Ionization and excitation of water molecules in intense laser pulses are studied theoretically by solving the three-dimensional time-dependent electronic Schrodinger equation within the single-active-electron approximation. The possibility to image orbital densities by measurement of the orientation-dependent ionization of H 2 O in few-cycle, 800 nm linear-polarized laser pulses is investigated. While the highest-occupied molecular orbital 1 b 1 is found to dominate the overall ionization behavior, contributions from the energetically lower lying 3 a 1 orbital dominate the ionization yield in the nodal plane of the 1 b 1 orbital. The ratio of the ionization yields of the two orbitals depends on the intensity. Furthermore, even for laser pulses as long as 8 cycles the orientation-dependent ion yield depends on the carrier-envelope phase. In the interpretation of the orientation-dependent ionization as an imaging tool these effects have to be considered." @default.
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- W2116049076 date "2013-03-01" @default.
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- W2116049076 title "Water molecules in ultrashort intense laser fields" @default.
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- W2116049076 doi "https://doi.org/10.1016/j.chemphys.2012.01.011" @default.
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