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- W2116203414 abstract "Abstract The exothermic, reversible formation of solid hydrides from the elements is rationalized on the basis of a model in which the hydride consists of hydrogen anions and metal cations, the latter likewise engaging in metal-metal bonding in the metallic hydrides. The lattice energy is evaluated as the sum of the Madelung energy and this metal-metal interaction energy. Two empirical methods of estimating the latter are suggested, one involving crystal field stabilization. The total lattice energy so calculated is compared semi-quantitatively with the sum of the endothermic factors in a Born-Haber cycle. The energy balance is favourable with few exceptions for hydrides known to form directly, and unfavourable for hydrides which evidently do not form directly from the elements." @default.
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- W2116203414 date "1962-04-01" @default.
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- W2116203414 title "A model for the rationalization of saline and metallic hydride formation" @default.
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- W2116203414 doi "https://doi.org/10.1016/0022-1902(62)80029-3" @default.
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