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- W2116522195 abstract "A novel synthetic route for preparation of amphiphilic heteroleptic ruthenium(II) complexes of the type [Ru(H2dcbpy)Cl(cymene)]NO3 (1) [Ru(H2dcbpy)(dmbpy)(NCS)2] (2), [Ru(H2dcbpy)(dhbpy)(NCS)2] (3) [Ru(H2dcbpy)(dnbpy)(NCS)2] (4) and [Ru(H2dcbpy)(dtdbpy)(NCS)2] (5) have been developed starting from dichloro(p-cymene)ruthenium(II) dimer. The performance of these complexes as charge-transfer photosensitizers in nanocrystalline TiO2-based solar cells was studied. When anchored complexes 2–5 onto a 12+4 μm thick nanocrystalline TiO2 films achieve very efficient sensitization over 85±5% incident photon-to-current efficiencies (IPCEs) in the visible region. Under standard AM 1.5 sunlight, using an electrolyte consisting of 0.6 M BMII; 0.05 M I2; 0.1 M LiI; 0.5 M tert-butyl pyridine in 1:1 acetonitrile + valeronitrile the films yielded a short circuit photocurrent density of 16±0.5 mA/cm2 and the open circuit voltage was 700±50 mV and a fill factor of 0.75±0.05, corresponding to an overall conversion efficiency of 8.6%. Solar cells based on amphiphilic sensitizers show remarkable stability under both thermal stress and light soaking matching the durability criteria applied to silicon solar cells for outdoor applications." @default.
- W2116522195 created "2016-06-24" @default.
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- W2116522195 date "2004-07-01" @default.
- W2116522195 modified "2023-10-10" @default.
- W2116522195 title "Stepwise assembly of amphiphilic ruthenium sensitizers and their applications in dye-sensitized solar cell" @default.
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- W2116522195 doi "https://doi.org/10.1016/j.ccr.2004.03.012" @default.
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