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• W2116726557 abstract "To surmount these obstacles, conventional PHJ PVSCs with the confi guration of substrate/HTL (p)/perovskite (i)/fullerene derivative (n) has been developed. [ 9 ] PEDOT:PSS or NiO X are the commonly employed HTLs to date while the electron-transporting layers (ETLs) employed are mainly based on fullerene derivatives. [ 7c,9c,d,10 ] It is worth noting that room temperature and orthogonal solvent processability of fullerene derivatives can successfully prevent the degradation of the underlying perovskite layer. In addition, the decent electron mobility of most fullerene derivatives makes them promising ETLs for high-performance PVSCs. Guo et al. fi rst demonstrated the feasibility of such a conventional PHJ confi guration, realizing a PCE of 3.9% by employing a phenyl-C 61 -butyric acid methyl ester (PC 61 BM) ETL. [ 9c ] Although three different fullerene derivatives (C 60 , PC 61 BM, and indene-C 60 bisadduct (IC 60 BA)) were investigated as ETLs, the functions of these fullerene-based interlayers were not fairly explored due to the inferior quality of the perovskite thin fi lm grown atop them. Soon after, a PC 61 BM ETL was used in a similar PHJ structure by Lam et al. to further improve the device performance to 7.4% by optimizing the perovskite precursor solution concentration and the blending ratio of PbI 2 and methylammonium iodide (MAI). [ 9a ] Lately, Jen and co-workers have signifi cantly enhanced the PCE to 12%–13%, respectively, by optimizing perovskite deposition either by controlling annealing conditions or adding a solvent additive.[11] Most recently, Seok and co-workers have reported an over 14% PCE through solvent engineering and thickness optimization of PC 61 BM. [ 12 ]" @default.
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• W2116726557 date "2015-02-27" @default.
• W2116726557 modified "2023-10-03" @default.
• W2116726557 title "Roles of Fullerene-Based Interlayers in Enhancing the Performance of Organometal Perovskite Thin-Film Solar Cells" @default.
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• W2116726557 doi "https://doi.org/10.1002/aenm.201402321" @default.
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