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• W2117060551 abstract "Abstract The vanadium‐dependent chloroperoxidase Mcl24 was discovered to mediate a complex series of unprecedented transformations in the biosynthesis of the merochlorin meroterpenoid antibiotics. In particular, a site‐selective naphthol chlorination is followed by an oxidative dearomatization/terpene cyclization sequence to build up the stereochemically complex carbon framework of the merochlorins in one step. Inspired by the enzyme reactivity, a chemical chlorination protocol paralleling the biocatalytic process was developed. These chemical studies led to the identification of previously overlooked merochlorin natural products." @default.
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• W2117060551 date "2014-08-21" @default.
• W2117060551 modified "2023-10-18" @default.
• W2117060551 title "A Multitasking Vanadium-Dependent Chloroperoxidase as an Inspiration for the Chemical Synthesis of the Merochlorins" @default.
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• W2117060551 doi "https://doi.org/10.1002/anie.201405696" @default.
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