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• W2117549452 abstract "Abstract Aryl‐ and heteroarylcyclobutenone rearrangements proceed in excellent yield under continuous‐flow conditions. The former shows a Hammett correlation with σ I providing strong evidence that electrocyclisation is the rate‐determining step and has a late transition state. The reaction has been modelled by using DFT and CCSD(T) methods, with the latter giving excellent correlation with the experimental rate constant. A short and efficient total synthesis of cribrostatin 6, an anti‐neoplastic and anti‐microbial agent, provides a topical demonstration of the value of this method." @default.
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• W2117549452 date "2011-11-14" @default.
• W2117549452 modified "2023-10-18" @default.
• W2117549452 title "New Insights into Cyclobutenone Rearrangements: A Total Synthesis of the Natural ROS-Generating Anti-Cancer Agent Cribrostatin 6" @default.
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• W2117549452 doi "https://doi.org/10.1002/chem.201102263" @default.
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