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• W2118073719 endingPage "8730" @default.
• W2118073719 startingPage "8723" @default.
• W2118073719 abstract "Abstract Lithium‐rich layer‐structured oxides x Li 2 MnO 3 ⋅ (1− x )LiMO 2 (0< x <1, M=Mn, Ni, Co, etc.) are interesting and potential cathode materials for high energy‐density lithium ion batteries. However, the characteristic charge compensation contributed by O 2− in Li 2 MnO 3 leads to the evolution of oxygen during the initial Li + ion extraction at high voltage and voltage fading in subsequent cycling, resulting in a safety hazard and poor cycling performance of the battery. Molybdenum substitution was performed in this work to provide another electron donor and to enhance the electrochemical activity of Li 2 MnO 3 ‐based cathode materials. X‐ray diffraction and adsorption studies indicated that Mo 5+ substitution expands the unit cell in the crystal lattice and weakens the LiO and MnO bonds, as well as enhancing the activity of Li 2 MnO 3 by lowering its delithiation potential and suppressing the release of oxygen. In addition, the chemical environment of O 2− ions in molybdenum‐substituted Li 2 MnO 3 is more reversible than in the unsubstituted sample during cycling. Therefore molybdenum substitution is expected to improve the performances of the Li 2 MnO 3 ‐based lithium‐rich cathode materials." @default.
• W2118073719 created "2016-06-24" @default.
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• W2118073719 date "2014-06-17" @default.
• W2118073719 modified "2023-10-18" @default.
• W2118073719 title "Molybdenum Substitution for Improving the Charge Compensation and Activity of Li₂MnO₃" @default.
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• W2118073719 doi "https://doi.org/10.1002/chem.201402727" @default.
• W2118073719 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24939463" @default.
• W2118073719 hasPublicationYear "2014" @default.
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