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- W2118253725 abstract "Abstract A qualitative PBC analysis of the COD structure results in five F forms: {110}, {101}, {100}, {121} and {211}. In order to quantify the morphological importance of these forms, their attachment energies are computed in an electrostatic point charge model. This model is derived for the oxalate ion from theoretical chemical considerations and simplified for the purpose to C 2 +1 O 4 -1 . The growth forms are constructed from the attachment energies, assumed to be proportional to the growth rates. Contrary to the observed morphology, the theoretical morphology is dominated by {110}. This discrepancy can be accounted for by noting that the elementary growth layer d 110 can be subdivided into two equivalent F slices with thickness 1 2 d 110 . Both have the same slice energy, which is furthermore smaller than the d 110 slice energy. When spiral and/or 2D growth mechanism occurs by means of both 1 2 d 110 F slices alternatingly in space and in time, the corresponding rate is higher than in the convential case of step thickness d 110 . The presence of this growth mechanism, viewed as an extension of the original PBC theory, leads to an improved theoretical morphology in better agreement with the observed one." @default.
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- W2118253725 date "1984-07-01" @default.
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- W2118253725 title "The theoretical growth morphology of calcium oxalate dihydrate" @default.
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