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• W2118713247 abstract "The structure of octadecanethiol monolyers on liquid Hg surfaces, measured with subangstrom resolution, evolves with increasing coverage from a laterally disordered phase of surface-parallel molecules to ordered rotator phases of surface-normal molecules. For the latter, an abrupt transition is found at $19text{ }text{ }{AA{}}^{2}/mathrm{text{molecule}}$ from a rectangular packing of molecules tilted by $27ifmmode^circelsetextdegreefi{}$ in the nearest-neighbor direction to a hexagonal unit cell of untilted molecules. The unit cell of the tilted phase is centered for the chains and noncentered for the headgroups. The thiol headgroups associate in pairs with a single Hg atom, and the bonds form long-range orientational order. The different order of thiols on Au(111) and on Hg highlights the subphase's role in determining the overlayer's structure." @default.
• W2118713247 created "2016-06-24" @default.
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• W2118713247 date "2005-01-12" @default.
• W2118713247 modified "2023-10-17" @default.
• W2118713247 title "Crystalline Phases of Alkyl-Thiol Monolayers on Liquid Mercury" @default.
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• W2118713247 doi "https://doi.org/10.1103/physrevlett.94.017802" @default.
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